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engine - 10:30 am on May 8, 2008 (gmt 0)
The dictionary and thesaurus, a book on the subject matter, coupled with sample searches, pulls up the majority of short and long tail terms, for me. Put your mind in the place of a prospective searcher.
The biggest problem with bought in databases is that the information is skewed by people checking on their own sites.
Go for phrases and terms that people would naturally type.